Coontz, R. & Hanson, B. Not so simple. Science 305, 957 (2004).
Barkai, E., Jung, Y. J. & Silbey, R. Theory of single-molecule spectroscopy: beyond the ensemble average. Annu. Rev. Phys. Chem. 55, 457–507 (2004).
Article CAS PubMed Google Scholar
Zrimsek, A. B. et al. Single-molecule chemistry with surface- and tip-enhanced Raman spectroscopy. Chem. Rev. 117, 7583–7613 (2017).
Article CAS PubMed Google Scholar
Lu, H. P., Xun, L. & Xie, X. S. Single-molecule enzymatic dynamics. Science 282, 1877–1882 (1998).
Article CAS PubMed Google Scholar
Liu, C. et al. Single polymer growth dynamics. Science 358, 352–355 (2017).
Article CAS PubMed Google Scholar
Florin, E. L., Moy, V. T. & Gaub, H. E. Adhesion forces between individual ligand-receptor pairs. Science 264, 415–417 (1994).
Article CAS PubMed Google Scholar
Li, Y., Yang, C. & Guo, X. Single-molecule electrical detection: a promising route toward the fundamental limits of chemistry and life science. Acc. Chem. Res. 53, 159–169 (2020).
Article CAS PubMed Google Scholar
Xin, N. et al. Concepts in the design and engineering of single-molecule electronic devices. Nat. Rev. Phys. 1, 211–230 (2019).
Venkatesan, B. M. & Bashir, R. Nanopore sensors for nucleic acid analysis. Nat. Nanotechnol. 6, 615–624 (2011).
Article CAS PubMed Google Scholar
Aviram, A. & Ratner, M. A. Molecular rectifiers. Chem. Phys. Lett. 29, 277–283 (1974).
Xiang, D., Wang, X., Jia, C., Lee, T. & Guo, X. Molecular-scale electronics: from concept to function. Chem. Rev. 116, 4318–4440 (2016).
Article CAS PubMed Google Scholar
Li, T., Hu, W. & Zhu, D. Nanogap electrodes. Adv. Mater. 22, 286–300 (2010).
Jia, C. & Guo, X. Molecule-electrode interfaces in molecular electronic devices. Chem. Soc. Rev. 42, 5642–5660 (2013).
Article CAS PubMed Google Scholar
Su, T. A., Neupane, M., Steigerwald, M. L., Venkataraman, L. & Nuckolls, C. Chemical principles of single-molecule electronics. Nat. Rev. Mater. 1, 16002 (2016).
Xu, B. & Tao, N. Measurement of single-molecule resistance by repeated formation of molecular junctions. Science 301, 1221–1223 (2003).
Article CAS PubMed Google Scholar
Venkataraman, L., Klare, J. E., Nuckolls, C., Hybertsen, M. S. & Steigerwald, M. L. Dependence of single-molecule junction conductance on molecular conformation. Nature 442, 904–907 (2006).
Article CAS PubMed Google Scholar
Reed, M. A., Zhou, C., Muller, C. J., Burgin, T. P. & Tour, J. M. Conductance of a molecular junction. Science 278, 252–254 (1997).
Park, H., Lim, A. K. L., Alivisatos, A. P., Park, J. & McEuen, P. L. Fabrication of metallic electrodes with nanometer separation by electromigration. Appl. Phys. Lett. 75, 301–303 (1999).
Park, J. et al. Coulomb blockade and the Kondo effect in single-atom transistors. Nature 417, 722–725 (2002).
Article CAS PubMed Google Scholar
Gehring, P. et al. Field-effect control of graphene–fullerene thermoelectric nanodevices. Nano Lett. 17, 7055–7061 (2017).
Article CAS PubMed Google Scholar
Burzurí, E. et al. Sequential electron transport and vibrational excitations in an organic molecule coupled to few-layer graphene electrodes. ACS Nano 10, 2521–2527 (2016).
Burzurí, E. et al. Spin-state dependent conductance switching in single molecule-graphene junctions. Nanoscale 10, 7905–7911 (2018).
Island, J. O. et al. Fabrication of hybrid molecular devices using multi-layer graphene break junctions. J. Phys. Condens. Matter 26, 474205 (2014).
Article CAS PubMed Google Scholar
Prins, F. et al. Room-temperature gating of molecular junctions using few-layer graphene nanogap electrodes. Nano Lett. 11, 4607–4611 (2011).
Article CAS PubMed Google Scholar
Lau, C. S. et al. Redox-dependent Franck–Condon blockade and avalanche transport in a graphene-fullerene single-molecule transistor. Nano Lett. 16, 170–176 (2015).
Limburg, B. et al. Anchor groups for graphene-porphyrin single-molecule transistors. Adv. Funct. Mater. 28, 1803629 (2018).
Mol, J. A. et al. Graphene-porphyrin single-molecule transistors. Nanoscale 7, 13181–13185 (2015).
Article CAS PubMed Google Scholar
Thomas, J. O. et al. Understanding resonant charge transport through weakly coupled single-molecule junctions. Nat. Commun. 10, 4628 (2019).
Article PubMed PubMed Central Google Scholar
Pei, T. et al. Exchange-induced spin polarization in a single magnetic molecule junction. Nat. Commun. 13, 4506 (2022).
Article CAS PubMed PubMed Central Google Scholar
Zhao, S. et al. Charge transport through single-molecule bilayer-graphene junctions with atomic thickness. Chem. Sci. 13, 5854–5859 (2022).
Article CAS PubMed PubMed Central Google Scholar
Cao, Y. et al. Building high-throughput molecular junctions using indented graphene point contacts. Angew. Chem. Int. Ed. Engl. 51, 12228–12232 (2012).
Article CAS PubMed Google Scholar
Gu, C. H., Su, D. K., Jia, C. C., Ren, S. Z. & Guo, X. F. Building nanogapped graphene electrode arrays by electroburning. RSC Adv. 8, 6814–6819 (2018).
Article CAS PubMed PubMed Central Google Scholar
Guo, X. et al. Covalently bridging gaps in single-walled carbon nanotubes with conducting molecules. Science 311, 356–359 (2006).
Article CAS PubMed Google Scholar
Jia, C. et al. Covalently bonded single-molecule junctions with stable and reversible photoswitched conductivity. Science 352, 1443–1445 (2016).
Article CAS PubMed Google Scholar
Jia, C., Ma, B., Xin, N. & Guo, X. Carbon electrode-molecule junctions: a reliable platform for molecular electronics. Acc. Chem. Res. 48, 2565–2575 (2015).
Article CAS PubMed Google Scholar
Xin, N. et al. Stereoelectronic effect-induced conductance switching in aromatic chain single-molecule junctions. Nano Lett. 17, 856–861 (2017).
Article CAS PubMed Google Scholar
Meng, L. et al. Atomically precise engineering of single-molecule stereoelectronic effect. Angew. Chem. Int. Ed. Engl. 60, 12274–12278 (2021).
Article CAS PubMed Google Scholar
Yang, C. et al. Complete deciphering of the dynamic stereostructures of a single aggregation-induced emission molecule. Matter 5, 1224–1234 (2022).
Wen, H. et al. Complex formation dynamics in a single-molecule electronic device. Sci. Adv. 2, e1601113 (2016).
Article PubMed PubMed Central Google Scholar
Zhou, C. et al. Direct observation of single-molecule hydrogen-bond dynamics with single-bond resolution. Nat. Commun. 9, 807 (2018).
Article PubMed PubMed Central Google Scholar
Liu, Z. et al. A single-molecule electrical approach for amino acid detection and chirality recognition. Sci. Adv. 7, eabe4365 (2021).
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